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ChemicalBook CAS DataBase List Carbamic acid, 3-furanyl-, 1,1-dimethylethyl ester (9CI)
56267-48-2

Carbamic acid, 3-furanyl-, 1,1-dimethylethyl ester (9CI) synthesis

2synthesis methods
-

Yield:56267-48-2 78%

Reaction Conditions:

with diphenyl phosphoryl azide;triethylamine in toluene at 20;Reflux;

Steps:

2.e
e. To a solution of 3-furoic acid 96 (54.4 g, 485 mmol), triethylamine (105 ml, 753 mmol), tert-butanol (25.2 mL, 786 mmol) in toluene (800 mL) was added dropwise at room temperature over 45 min period diphenyl phosphoryl azide (157.8 mL, 732 mmol). The resulting solution was heated at reflux for 6 h and at room temperature overnight. The reaction was diluted with water (1000 mL) and extracted twice with ethyl acetate (1000 ml). The organic layers were combined washed with water (800 mL), brine (800 mL), decolorized with activated charcoal, dried, filtered and concentrated in vacuo to furnish a brown semisolid. The semisolid was crystallized from dichloromethane (300 mL) and hexanes (600 mL) to furnish tert-butyl furan-3-ylcarbamate 97 (61.5 g, 78%). 1H NMR (300 MHz, CDC13) δ 7.71 (s, IH), 7.30 - 7.24 (m, IH), 6.43 (s, IH), 6.27 (s, IH), 1.75 - 1.32 (s, 9H).

References:

BIOCRYST PHARMACEUTICALS, INC.;BABU, Yarlagadda, S.;CHAND, Pooran;KOTIAN, Pravin, L.;KUMAR, V., Satish WO2010/14930, 2010, A2 Location in patent:Page/Page column 39

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