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ChemicalBook CAS DataBase List 2,6-Difluorophenylboronic acid
162101-25-9

2,6-Difluorophenylboronic acid synthesis

4synthesis methods
-

Yield: 27 g

Reaction Conditions:

Stage #1:1,3-Difluorobenzene with n-butyllithium in diethyl ether;hexane at -70 - -60; for 2 h;Inert atmosphere;
Stage #2:Trimethyl borate in diethyl ether;hexane at -60 - -50; for 2 h;Inert atmosphere;Reagent/catalyst;Temperature;Solvent;

Steps:

1
500 ml of dry reaction flask was replaced with nitrogen, 22.8 g of compound (1), 150 ml of anhydrous ether Liter, and the system was cooled to -78 ° C under nitrogen. The mixture was slowly added dropwise with 187 ml of 1.6 M n-hexane solution of n-butyllithium. After the addition, the reaction was stirred at -60 to -70 ° C 2 hours. The system was re-cooled to -78 ° C, dropping 60 grams of trimethyl borate, dropping finished, the control temperature -50 ~ -60 ° C stirring reaction 2 hours. The reaction was warmed to room temperature, 200 ml of water was added to quench the reaction, and the mixture was acidified with 36% hydrochloric acid. After the organic solvent was recovered by distillation at elevated temperature, the reaction was stirred at 70 to 80 ° C for 6 hours. The system was cooled to crystallize, filtered and washed with water to obtain 27.0 g of the compound (II)

References:

ZHEJIANG ZHONGXIN FU CAI CO LTD/ ZHEJIANG ZHONGXIN CHEMICALS CO., LTD.;YUAN, QILIANG;ZHANG, JIABING;XU, PENGFEI;JIANG, XIANBO;CHEN, YINHAO;WANG, CHAO CN103819401, 2016, B Location in patent:Paragraph 0023; 0066; 0067

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